Tim Buckley, “Live at the Folklore Center, NYC, March 6, 1967”; released in 2009.
The first time I listened through this last week, I didn’t pay attention to the date and thought he sounds like he’s going for a sound like 1960s folk. And then I looked at the date of the concert and realized that he wasn’t "going for" it, he was in it. Think early Bob Dylan. Particularly striking song on this album: “No Man Can Find the War.